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Journal Articles

Muon spin relaxation in mixed perovskite (LaAlO$$_3$$)$$_x$$(SrAl$$_{0.5}$$Ta$$_{0.5}$$O$$_3$$)$$_{1-x}$$ with $$xsimeq 0.3$$

Ito, Takashi; Higemoto, Wataru; Koda, Akihiro*; Nakamura, Jumpei*; Shimomura, Koichiro*

Interactions (Internet), 245(1), p.25_1 - 25_7, 2024/12

JAEA Reports

Thermal-hydraulic design calculations for JRR-3 cold neutron source with the new moderator cell

Tokunaga, Sho; Horiguchi, Hironori; Nakamura, Takemi

JAEA-Technology 2023-001, 37 Pages, 2023/05

JAEA-Technology-2023-001.pdf:1.39MB

The cold neutron source (CNS) of the research reactor JRR-3 converts thermal neutrons generated in the reactor into low-energy cold neutrons by moderating them with liquid hydrogen stored in the moderator cell. Cold neutrons generated by the CNS are transported to experimental instruments using neutron conduits, and are used for many studies of physical properties, mainly in life science, polymer science, environmental science, etc. Improvement of cold neutron intensity is essential to maintain competitiveness with the world's research reactors in neutron science, and we are developing a new CNS that incorporates new knowledge. The current moderator cell for the CNS of JRR-3 is a stainless-steel container which is a canteen bottle type, and the cold neutron intensity can be improved by changing the material and shape. Therefore, the basic specifications of the new moderator cell were changed to aluminum alloy which has a smaller neutron absorption cross section, and the shape was optimized using a Monte Carlo code MCNP. Since these changes in specifications will result in changes in heat generation and heat transfer conditions, the CNS of JRR-3 was re-evaluated in terms of self-regulating characteristic, heat transport limits, heat resistance and pressure resistance, etc., to confirm its feasibility in thermal-hydraulic design. This report summarizes the results of the thermal-hydraulic design evaluation of the new moderator cell.

Journal Articles

Effectiveness evaluation methodology of the measures for improving resilience of nuclear structures against excessive earthquake

Kurisaka, Kenichi; Nishino, Hiroyuki; Yamano, Hidemasa

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 8 Pages, 2023/05

The objective of this study is to develop an effectiveness evaluation methodology of the measures for improving resilience of nuclear structures against excessive earthquake by applying the failure mitigation technology. This study regarded those measures for improving resilience of important structures, systems, and components for safety to enlarge their seismic safety margin. To evaluate effectiveness of those measures, seismic core damage frequency (CDF) is selected as an index. Reduction of CDF as an effectiveness index is quantified by applying seismic PRA technology. Accident sequences leading to loss of decay heat removal are significant contributor to seismic CDF of sodium-cooled fast reactors (SFRs), and those sequences result in core damage via ultra-high temperature condition. This study improved the methodology to evaluate not only the measures against shaking due to excessive earthquake but also the measures at the ultra-high temperature condition. To examine applicability of the improved methodology, a trial calculation was implemented with some assumptions for a loop-type SFR. Within the assumption, the measures for improving resilience were significantly effective for decreasing CDF in excessive earthquake up to several times of a design basis ground motion. Through the applicability examination, the methodology for the effectiveness evaluation was developed successfully.

Journal Articles

Effectiveness evaluation methodology of the measures for improving resilience of nuclear structures at ultra-high temperature

Onoda, Yuichi; Kurisaka, Kenichi; Yamano, Hidemasa

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 7 Pages, 2023/05

The objective of this study is to develop an effectiveness evaluation methodology of the measures for improving resilience of nuclear structures at ultra-high temperature by using the failure mitigation technology. At the beginning, to identify the accident sequences having the potential to improve resilience, the characteristics of a next-generation loop-type sodium-cooled fast reactor (SFR) in Japan has been investigated by analyzing the event tree of level-1 and level-2 probabilistic risk assessment. As a result, event sequences of loss of heat removal systems (LOHRS) are identified. The effectiveness of the measures for improving resilience is evaluated by quantifying the reduction rate of core damage frequency before and after the introduction of the measures for improving resilience for all the accident sequences leading to LOHRS. To examine applicability of the developed methodology, a trial evaluation has conducted for a next-generation loop-type SFR in Japan. Through the applicability examined, the method for the effectiveness evaluation was developed successfully. The refinement of the conditional success probability of the measures for improving resilience is the future work.

Journal Articles

Engineering formulation of the irradiation growth behavior of zirconium-based alloys for light water reactors

Kakiuchi, Kazuo; Amaya, Masaki; Udagawa, Yutaka

Journal of Nuclear Materials, 573, p.154110_1 - 154110_7, 2023/01

 Times Cited Count:0 Percentile:0.01(Materials Science, Multidisciplinary)

Journal Articles

On the adsorption and reactivity of element 114, flerovium

Yakushev, A.*; Lens, L.*; D$"u$llmann, Ch. E.*; Khuyagbaatar, J.*; J$"a$ger, E.*; Krier, J.*; Runke, J.*; Albers, H. M.*; Asai, Masato; Block, M.*; et al.

Frontiers in Chemistry (Internet), 10, p.976635_1 - 976635_11, 2022/08

 Times Cited Count:9 Percentile:79.28(Chemistry, Multidisciplinary)

Flerovium (Fl, element 114) is the heaviest element chemically studied so far. The first chemical experiment on Fl suggested that Fl is a noble-gas-like element, while the second studies suggested that Fl has a volatile-metal-like character. To obtain more reliable conclusion, we performed further experimental studies on Fl adsorption behavior on Si oxide and gold surfaces. The present results suggest that Fl is highly volatile and less reactive than the volatile metal, Hg, but has higher reactivity than the noble gas, Rn.

Journal Articles

Irradiation growth behavior and effect of hydrogen absorption of Zr-based cladding alloys for PWR

Kakiuchi, Kazuo; Amaya, Masaki; Udagawa, Yutaka

Annals of Nuclear Energy, 171, p.109004_1 - 109004_9, 2022/06

 Times Cited Count:4 Percentile:78.52(Nuclear Science & Technology)

Journal Articles

Detection of Simulated Fukushima Daiichi Fuel Debris Using a Remotely Operated Vehicle at the Naraha Test Facility

Nancekievill, M.*; Espinosa, J.*; Watson, S.*; Lennox, B.*; Jones, A.*; Joyce, M. J.*; Katakura, Junichi*; Okumura, Keisuke; Kamada, So*; Kato, Michio*; et al.

Sensors (Internet), 19(20), p.4602_1 - 4602_16, 2019/10

 Times Cited Count:7 Percentile:38.52(Chemistry, Analytical)

In order to contribute to fuel debris search at the Fukushima Daiichi Nuclear Power Station, we developed a system to search for submerged fuel debris by mounting a sonar on the remotely operated vehicle (ROV). The system can obtain 3D images of submerged fuel debris in real time by using the positioning system, depth sensor, and collected sonar data. As a demonstration test, a simulated fuel debris was installed at the bottom of the water tank facility at the Naraha Center for Remote Control Technology Development, and a 3D image was successfully obtained.

Journal Articles

Irradiation growth behavior of improved Zr-based alloys for fuel cladding

Amaya, Masaki; Kakiuchi, Kazuo; Mihara, Takeshi

Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.1048 - 1056, 2019/09

Journal Articles

Development of ROV system to explore fuel debris in the Fukushima Daiichi Nuclear Power Plant

Kamada, So*; Kato, Michio*; Nishimura, Kazuya*; Nancekievill, M.*; Watson, S.*; Lennox, B.*; Jones, A.*; Joyce, M. J.*; Okumura, Keisuke; Katakura, Junichi*

Progress in Nuclear Science and Technology (Internet), 6, p.199 - 202, 2019/01

As a technology development to investigate the distribution of submerged fuel debris in the primary containment vessel (PCV) of the Fukushima Daiichi Nuclear Power Station, we are conducting development experiments of sonar system to be mounted in a compact ROV. The experiments were conducted in two types of water tanks with different depths, simulating the PCV, using sonar with different sizes, ultrasonic frequencies, and beam scanning method, and simulated fuel debris. As a result, we characterized the shape discrimination performance of the simulated debris, and the noise due to multi-path in narrow closed space.

Journal Articles

Online chemical adsorption studies of Hg, Tl, and Pb on SiO$$_{2}$$ and Au surfaces in preparation for chemical investigations on Cn, Nh, and Fl at TASCA

Lens, L.*; Yakushev, A.*; D$"u$llmann, Ch. E.*; Asai, Masato; Ballof, J.*; Block, M.*; David, H. M.*; Despotopulos, J.*; Di Nitto, A.*; Eberhardt, K.*; et al.

Radiochimica Acta, 106(12), p.949 - 962, 2018/12

AA2018-0417.pdf:0.99MB

 Times Cited Count:8 Percentile:62.99(Chemistry, Inorganic & Nuclear)

Online gas-solid adsorption studies with single atom quantities of Hg, Tl, and Pb on SiO$$_{2}$$ and Au surfaces were carried out using short-lived radioisotopes with half-lives in the range of 4-49 s. This is a model study to measure adsorption enthalpies of superheavy elements Cn, Nh, and Fl. The short-lived isotopes were produced and separated by the gas-filled recoil separator TASCA at GSI. The products were stopped in He gas, and flushed into gas chromatography columns made of Si detectors whose surfaces were covered by SiO$$_{2}$$ or Au. The short-lived Tl and Pb were successfully measured by the Si detectors with the SiO$$_{2}$$ surface at room temperature. On the other hand, the Hg did not adsorb on the SiO$$_{2}$$ surface, but adsorbed on the Au surface. The results demonstrated that the adsorption properties of short-lived Hg, Tl, and Pb could be studied with this setup, and that this method is applicable to the experiment for Cn, Nh, and Fl.

Journal Articles

Behaviors of high-burnup LWR fuels with improved materials under design-basis accident conditions

Amaya, Masaki; Udagawa, Yutaka; Narukawa, Takafumi; Mihara, Takeshi; Taniguchi, Yoshinori

Proceedings of Annual Topical Meeting on Reactor Fuel Performance (TopFuel 2018) (Internet), 10 Pages, 2018/10

JAEA Reports

Petrographic data of silicic igneous rocks in the Tono area, central Japan

Ueki, Tadamasa; Niwa, Masakazu

JAEA-Data/Code 2018-005, 94 Pages, 2018/08

JAEA-Data-Code-2018-005.pdf:15.6MB

Mountain development has an influence on long-term changes of uplift, erosion, and groundwater flow related to change in hydraulic gradient. Provenance analysis is one of promising geological methods to understand origin and formation process of mountains. Case study in the Tono area, central Japan has been done for research and development of individual technique to estimate a provenance. In this report, petrological descriptions by meso- and microscopic observations and elemental distributions using scanning X-ray analytical microscope of basement rocks (silicic igneous rocks) from the study area were compiled.

Journal Articles

Thermal-hydraulics technological strategy roadmap 2017; An Approach for continuous safety improvement of LWRs

Itoi, Tatsuya*; Iwaki, Chikako*; Onuki, Akira*; Kito, Kazuaki*; Nakamura, Hideo; Nishida, Akemi; Nishi, Yoshihisa*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 60(4), p.221 - 225, 2018/04

no abstracts in English

Journal Articles

Polar rotor scattering as atomic-level origin of low mobility and thermal conductivity of perovskite CH$$_{3}$$NH$$_{3}$$PbI$$_{3}$$

Li, B.; Kawakita, Yukinobu; Liu, Y.*; Wang, M.*; Matsuura, Masato*; Shibata, Kaoru; Kawamura, Seiko; Yamada, Takeshi*; Lin, S.*; Nakajima, Kenji; et al.

Nature Communications (Internet), 8, p.16086_1 - 16086_9, 2017/06

 Times Cited Count:81 Percentile:91.64(Multidisciplinary Sciences)

Journal Articles

Challenges for enhancing Fukushima environmental resilience, 2; Features of radionuclide release and deposition with accident progress

Saito, Kimiaki; Nagai, Haruyasu; Kinase, Sakae; Takemiya, Hiroshi

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 59(6), p.40 - 44, 2017/06

no abstracts in English

Journal Articles

A Remote-operated system to map radiation dose in the Fukushima Daiichi primary containment vessel

Nancekievill, M.*; Jones, A. R.*; Joyce, M. J.*; Lennox, B.*; Watson, S.*; Katakura, Junichi*; Okumura, Keisuke; Kamada, So*; Kato, Michio*; Nishimura, Kazuya*

Proceedings of 5th International Conference on Advancements in Nuclear Instrumentation Measurement Methods and their Applications (ANIMMA 2017) (USB Flash Drive), 6 Pages, 2017/06

We are developping a submersible ROV system, coupled with radiation detectors aimed at mapping the interior of the reactors at the Fukushima Daiichi Nuclear Power Station. To map the $$gamma$$-ray intensity environment a cerium bromide (CeBr$$_{3}$$) inorganic scintillator detector sensitive to $$gamma$$-rays has been incorporated into the ROV to measure $$gamma$$-ray intensity and identify radioactive isotopes. The ROV is a cylindrical shape with a diameter of about 150 mm, and it have two end caps of five pumps each allowing control of the ROV in 5 degree of freedom. It is possible to directly replace the CeBr$$_{3}$$ detector with a single crystal chemical vapour deposition (CVD) neutron detector with a $$^{6}$$Li convertor foil that is capable of mapping the thermal neutron flux.

Journal Articles

Thermal-hydraulics technological strategy roadmap that improves safety of LWRs

Arai, Kenji*; Umezawa, Shigemitsu*; Oikawa, Hirohide*; Onuki, Akira*; Nakamura, Hideo; Nishi, Yoshihisa*; Fujii, Tadashi*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 58(3), p.161 - 166, 2016/03

no abstracts in English

Journal Articles

Thermophysical properties of americium-containing barium plutonate

Tanaka, Kosuke; Sato, Isamu; Hirosawa, Takashi; Kurosaki, Ken*; Muta, Hiroaki*; Yamanaka, Shinsuke*

Journal of Nuclear Science and Technology, 52(10), p.1285 - 1289, 2015/10

 Times Cited Count:2 Percentile:17.57(Nuclear Science & Technology)

Polycrystalline specimens of americium-containing barium plutonate have been prepared by mixing the appropriate amounts of (Pu$$_{0.91}$$Am$$_{0.09}$$)O$$_{2}$$ and BaCO$$_{3}$$ powders followed by reacting and sintering at 1600 K under the flowing gas atmosphere of dry-air. The sintered specimens had a single phase of orthorhombic perovskite structure and were crack-free. The elastic moduli were determined from the longitudinal and shear sound velocities. The Debye temperature was also determined from the sound velocities and lattice parameter measurements. The thermal conductivity was calculated from the measured density at room temperature, literature values of heat capacity, and thermal diffusivity measured by laser flash method in vacuum. The thermal conductivity of americium-containing barium plutonate was roughly independent of the temperature and was almost the same magnitude as that of BaPuO$$_{3}$$ and BaUO$$_{3}$$.

Journal Articles

Primary radiation damage in materials

Nordlund, K.*; Sand, A. E.*; Granberg, F.*; Zinkle, S. J.*; Stoller, R.*; Averback, R. S.*; Suzudo, Tomoaki; Malerba, L.*; Banhart, F.*; Weber, W. J.*; et al.

NEA/NSC/DOC(2015)9 (Internet), 86 Pages, 2015/00

Within this report, we review the current understanding of primary radiation damage from neutrons, ions and electrons with emphasis on the range of validity of the dpa concept in all main classes of materials, and in particular discuss known shortcomings. We recognise that the current NRT-dpa standard is fully valid in the sense of a scaled radiation exposure measure, as it is essentially proportional to the radiation energy deposited per volume. As such, it is highly recommended to be used in reporting neutron damage results to enable comparison between different nuclear reactor environments and ion irradiations. However, in the sense of a measure of damage production the NRT-dpa value has several well-known problems. We discuss this matter and propose an improved dpa definition.

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